Without a doubt bone. The order of sonic improvement upgrades I THINK are as follows:
1) Saddle
2) Pins
3) Nut
Whether pins and nut make a discernable difference is definitely a subject of debate, but from where I sit they are both a relatively inexpensive upgrade and they certainly can't hurt. Also, as far as the nut goes, bone will definitely last much longer and won't need to be fixed or filed as it won't ever develop sharp spots.
I'd say got for them all! You won't break the bank and they can only help so why not?
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