Polyweb's have a thicker coating and seem to damp down on the brightness a fair bit, so this may affect volume. I think the nanoweb light's are better on the baby.
I also tried mediums on the baby once but it didn't really sound right, nanoweb lights seem to make the guitar ring best. I think the general view is that these strings along with a low action minimise intonation issues on the guitar. Medium strings also can be too much for the neck over time.
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